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Information about source points of anthropogenic radioactivity
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|
SECTION 11: ANTHROPOGENIC RADIOACTIVITY: MAJOR PLUME SOURCE
POINTS
|
Except the Chernobyl nuclear power plant accident of April
26, 1986: See RAD 10
Table of Contents
-
Introduction
-
General Bibliography
-
Nuclear Weapons Test Explosions
A. Marshall Islands
B. Johnston Atoll
-
Nuclear Power Plants
A. United States Nuclear
Power Plants
-
Maine Yankee
-
Connecticut Yankee
-
Three Mile Island
-
Other Citations about U.S. Nuclear Power
Plants
-
Safety Issues at U.S. Nuclear Power Plants
a. Reactor Embrittlement
b. Spent Fuel Cladding Failure
c. Steam Generator Degradation
Mechanisms
d. LORCAs and Spent Fuel Cooling
e. Hot Particles
f. Spent Fuel Storage and
Disposal (Dry Casks/Multi Purpose Casks, etc.)
g. MOX
-
Nuclear Regulatory Commission Publications
(if not listed in any of the above categories)
B. Canadian Nuclear Power Plants
C. Russian Nuclear
Power Plants
D. Japanese Nuclear Power Plants
E. European Nuclear Power Plants
G. Biological Monitoring
(see extensive citations in RAD7: Plume Pulse Pathways)
-
United
States Military Source Points
A. U.S.
Military: General Bibliography
-
The Plutonium enigma
-
The Plutonium enigma:
Part 2
-
Deepwell Injection
B. U.S. Military: Specific Source Points
-
Argonne National Laboratory
-
Fernald, Ohio
-
Hanford Reservation, Washington
State
-
Idaho National
Engineering Laboratory
-
Lawrence
Livermore National Laboratory
-
Los Alamos National
Laboratory
-
Maxey Flats, Kentucky
-
Moab, Utah
-
Mound Laboratory,
Miamisburg, Ohio
-
Midwest Fuel
Recovery Plant (MFRP), Morris, Illinois
-
Nevada Test Site
-
Oak Ridge
National Laboratory, Tennessee
-
Pantex, Amarillo, Texas
-
Rocky Flats, Colorado
-
Sandia National Laboratories, New Mexico
-
Savannah River Plant, S.
Carolina
-
West Valley, New York
-
Russian Military
Source Points
-
Kyshtym 1957
-
Karachay Lake Wind Transfer
-
Techa River
-
Chelyabinsk
-
Kola Peninsula
-
Krasnoyarsk
-
Novaya Zemlya Test Site
-
Semipalatinsk Test Site
-
Tomsk
-
Sosnovyy Bor
-
Vladivostok
-
United
Kingdom Source Points
-
Dounreay
-
Sellafield
(Windscale) Fuel Reprocessing Facility
-
Marine Radioactive
Waste Dump Sites
-
Russian Ocean Dumping Sites
-
Nuclear Submarine
Accidents and Dump Sites
-
Nuclear
Powered Satellite Accidents
-
Uranium
Mining, Milling, and Processing
-
Depleted Uranium
-
Sealed Sources, Devices and
Radioactive Scrap
-
SNAP Power
Generators
-
Scrap Metal
-
Medical
-
Food and Irradiation
-
Industrial Measuring
-
Other
-
Other
Important Foreign and Miscellaneous Source Points
-
French and Israeli Military
Source Points
-
Canadian Source Points
-
Cap de la Hague
-
Goiania, Brazil
-
Palomares, Spain
-
Rosyth, United Kingdom
-
Thule, Greenland
-
Sabotage and Terrorism
-
Missing Weapons Production
High-Level Waste
-
Sewage Sludge
-
The cumulative deposition in a wide mid-latitude band
of the northern hemisphere of weapons testing derived 239,240Pu
is now ~50 Bq/m2 (3,000 d.p.m./m2); testing derived
137Cs
exceeding 1,000 Bq/m2 remains in many locations. Other long-lived
radionuclides accompany these isotopes, some "growing in" as daughter products
from inert gases; others such as 241Am "grow in" as daughter
products of more dangerous isotopes such as 241Pu. The following
activities, facilities, and locations are either (or both) past or future
potential source points of the release of radioactivity into the environment,
in some cases with the potential for the dispersion of anthropogenic radioactivity
approaching or equaling the magnitude of the Chernobyl accident release.
-
The following citations are not intended to be a comprehensive
list, only a representative selection of research on the most important
past, present or potential contamination source points.
-
RADNET will shortly include a file pertaining to the mining,
milling and processing of uranium in the nuclear weapons production cycle;
RADNET includes little or no information about many other potential industrial
sources of radioactive contamination such as medical technology, food irradiation
equipment, etc.
-
Some topics are almost entirely omitted due to space limitations
or lack of data; e.g. research on European nuclear power and fuel reprocessing
facilities (the citations on Sellafield represent less than 1% of the available
literature on this topic), or information pertaining to French, Israeli
or Chinese weapons or nuclear power production.
-
The following annotated bibliography is a draft that will
be continually updated. RADNET readers are requested to provide any additional
citations or information about any of the plume source points discussed
in this section.
Memo: One PBq = 1x 1015 disintegration's per
second (Becquerels) = 27,000 Curies. With world wide inventories of spent
fuel and weapons production high-level wastes now approaching 100 billion
curies, use of the prefixes "P" (peta: 1015) and "E" (exo: 1018)
to describe becquerels of waste is unwieldy and misleading. Expressing
100 billion curies of high-level waste as 3,700 EBq is not only absurd,
it obfuscates the significance and the presence of these contained and
uncontained wastes, especially for lay persons who are likely to suffer
from psychic numbing while trying to differentiate the orders of magnitude
implied by M,E,G,P,T. RADNET readers who can assign the proper order of
magnitude to these letters without looking them up in RADNET Section 4,
please send a postcard to the Center for Biological Monitoring: if you
visit Mount Desert Island we will award you a free day pass to Acadia National
Park. |
Aarkrog, A., Botter-Jensen, L., Chen Qing Jang, Dahlgaard,
H., Hansen, H., Holm E., Lauridsen, B., Nielsen, S.P. and Sogaard-Hansen,
J. (1991). Environmental radioactivity in Denmark in 1988 and 1989.
Riso-R-570. Riso National Laboratory, Roskilde, Denmark.
Aarkrog, A. (1992). Source terms and inventories
of anthropogenic radionuclides. Report No. DK-4000. Riso National Laboratory,
Roskilde, Denmark.
-
In addition to 137Cs, 90Sr and
131I,
Aarkrog lists the following fission products as worthy of monitoring:
Sr-89, Y-91, Zr-95, Nb-95, Tc-99, Ru-103, Ru-106,
Sb-125, I-131, I-129, Cs-136, Ba-140, Ce-141, Ce-144, Eu-154, Eu-155.
-
This report is cited frequently in the following parts
of this section of RADNET.
Aarkrog, A., Botter-Jensen, L., Jiang, Chen Quing, Dahlgaard,
H., Hansen, H., Holm, E., Lauridsen, B., Nielsen, S.P., Strandberg, M.
and Sogaard-Hansen, J. (1992). Environmental radioactivity in Denmark
in 1990 and 1991. Riso National Laboratory, Roskilde, Denmark.
Aarkrog, A., Dahlgaard, H., Frissel, M., Foulquier, L.,
Kulikov, N.V., Molchanova, I.V., Myttenaere, C., Nielsen, S.P., Polikarpov,
G.G. and Yushkov, P.I. (1992). Sources of Anthropogenic Radionuclides in
the Southern Urals. J. Environ. Radioactivity, 15, pg. 69-80.
-
"...the southern Urals have significant sources of radioactive
contamination other than those officially reported. This fact may have
an impact on the global inventories of 90Sr and
137Cs."
(pg. 69).
-
"It is concluded that two sets of soil samples collected
in the Sverdlovsk region by a joint USSR-IUR expedition in May 1990 suggest
the presence of radioactive debris from (at least) four sources of contamination:
global fallout, the Kyshtym accident in 1957, the Chernobyl accident in
1986 and unreported releases from nuclear activities in the southern Urals,
probably the release from Lake Karachay in 1967." (pg. 79).
-
See Part 6 of this Section on Russian
military source points for more information on this topic.
Aarkrog, A., Tsaturov, Y. and
Polikarpov, G.G. (1993).
Sources to environmental radioactive contamination
in the former USSR. Riso National Laboratory, Roskilde, Denmark.
-
This report is a more detailed analysis of Soviet military
source points of radioactive contamination of the environment, but documents
only a tiny percentage of cold war era high-level wastes resulting from
Soviet military activities.
-
This report is also cited frequently in the following
parts of this section of RADNET.
Aarkrog, A. (1994). Radioactivity in polar regions - Main
sources. J. Environ. Radioactivity, 25, pg. 21-35.
-
Table 1: Inventory Estimates for Uncontained Radionuclides in the Polar
Regions (PBq) 1993 Estimates (p. 28).
-
A bioregional survey of uncontained releases of radioactivity,
the principal sources of Arctic contamination being Sellafield (15 PBq
137Cs),
global fallout (4.1 PBq), USSR river discharges (5 PBq), and Chernobyl
(5 PBq); all equal Aarkrog's highest estimates. Estimates of 90Sr
are approximately a third of the
137Cs estimates.
-
This is one of the many comprehensive reports from the
Riso National Laboratory in Denmark which will be cited throughout this
section of RADNET.
-
Total fallout in this bioregion estimated at 33 PBq of
137Cs
(892,000 curies). The polar regions are well away from the mid-latitude
regions which have received the highest level of weapons and Chernobyl
derived contamination.
-
Table 2: Lists preliminary estimates for other sources of radioactive
contamination of the Arctic (p. 29):
-
Komsomolet submarine, Barents Sea 1989 (Petrov, 1991): 2.9 PBq 90Sr,
3.1 PBq 137Cs
-
Sr-90 powered Lighthouses, Siberian coast (Aarkrog et al., 1994): 10-15
PBq 90Sr per unit
-
Dumped submarines at Novaya Zemlya (Yablokov et al., 1993): ~85 PBq
90Sr
and 137Cs
Aarkrog, A., Bøtter-Jensen, L., Chen Qing Jiang,
Clausen, J., Dahlgaard, H., Hansen, H., Holm, E., Lauridsen, B., Nielsen,
S.P., Strandberg, M. and Søgaard-Hansen, J. (1995). Environmental
radioactivity in Denmark in 1992 and 1993. Risø-R-756(EN). Riso
National Laboratory, Roskilde, Denmark.
Albright, D., Berkhout, F. and Walker, W. (1993). World
inventory of plutonium and highly enriched uranium, 1992. Oxford University
Press, Oxford.
Borson, D. et. al. (1990). Payment due: a reactor-by-reactor
assessment of the nuclear industry's $25+ billion decommissioning bill.
Public Citizen's Critical Mass Energy Project. Washington, DC. pp. 88.
Broden, K., Carugati, S., Brodersen, K., Carlsson,
T., Viitanen, P., Walderhaug, T., Sneve, M., Hornkjol, S., and Backe, S.
(November 18, 1997). Characterisation of long-lived low and intermediate-level
radioactive wastes in the nordic countries. NKS/AFA (97)8. Riso National
Laboratory, Roskilde, Denmark.
Burke, P., Ed. (1988). The nuclear weapons world:
Who, how & where. Oxford Research Group, London.
Cochran, T.B., Arkin, W.M., Norris, R.S. and Hoenig,
M.M. (1987). Nuclear Weapons Databook. Vol. 3, U.S. nuclear warhead
facilities profiles. Ballinger Publishing Company, Cambridge, Massachusetts.
Davis, M.D. (1988). The military-civilian nuclear
link: A guide to the French nuclear industry. Westview Press, Boulder,
Colorado.
de la Court, T., Pick, D. and Nordquist, D. (1982).
The
nuclear fix: a guide to nuclear activities in The Third World. WISE
Publications, Amsterdam.
DiNunno, Joseph J. (June 1997). Integrated
safety management. DNFSB/TECH-16. Defense Nuclear Facilities Safety
Board, Washington, D.C.
Eisenbud, M. and Gesell, T. (1997). Environmental
radioactivity: from natural, industrial, and military sources. Fourth
edition. Academic Press, San Diego, CA.
-
This is the fourth edition of one of the most comprehensive information
sources on environmental radioactivity.
-
This text is environmental radioactivity through rose colored glasses:
compare Eisenbud's comments on the relative harmlessness of plutonium in
Chapter 16 with Goffman's in Radiation and Human Health.
-
The misinformation about the Chernobyl source term in the 3rd edition
has been corrected (see chapter 12). No mention is made of the recent National
Cancer Institute report on 131I exposure during the 1950's
and 1960's which effectively deconstructs the traditional and beloved pie
chart (pg. 528) of exposure to sources of ionizing radiation (see RADNET
13: RADLINKS Part II-C: Health Physics Links).
-
Chapter 3 is an excellent survey of the chaotic world of radiation protection
guidelines. See also Chapter 16.
-
This fourth edition was published in 1997, but it is already out-of-date.
There is no reference to derived concentration guideline levels (DCGLs),
to the MARSSIM or to the FDA derived intervention level (DIL) guidelines
for contaminated foods.
-
Though containing some discussion of pathway exposure, this edition
contains only the briefest discussion of the recent changes from a concentration-based
to dose-based site release criteria as defined in MARSSIM.
-
If careful pathway analyses of long-lived spent fuel wastes (LLSFW)
is essential to establish credible TEDEs, one would not know it from reading
this important text.
Feshbach, M. and Friendly, Jr., A. (1992). Ecocide
in the USSR. Basic Books, New York.
International Atomic Energy Agency. (1971). Disposal
of radioactive wastes into rivers, lakes and estuaries. (Safety Series
No. 36). IAEA, Vienna.
-
One of the many publications of the IAEA, RADNET does
not have a copy of this text available for review and annotation. RADNET
readers are alerted to the many excellent but difficult to locate publications
of the IAEA, some of which are cited in RAD: 14, General Bibliography.
Most IAEA publications can be accessed by surfing the IAEA websites in
RAD: 13, RADLINKS. Even though the IAEA led the way in the ritual of aversion
pertaining to Chernobyl derived fallout patterns, an as a subsidiary of
the United Nations has many of the qualities associated with ostriches,
the importance of the research in IAEA publications such as Transuranian
Nuclides in the Environment (1976) should not be underestimated.
International Joint Commission. (December 1997). Inventory
of radionuclides for the Great Lakes. Nuclear Task Force of the
International Joint Commission. Washington, DC.
-
Revised monitoring and analysis protocols are needed to assess how natural
and man-made radionuclides affect the ecosystem health. The inventory is
a first step in establishing the sources, pathways, distribution and movement
of radionuclides.
International Physicians for the Prevention of Nuclear
War (IPPNW). (1991). Radioactive Heaven and Earth. A Report
of the International Physicians for the Prevention of Nuclear War International
Commission to Investigate the Health and Environmental Effects of Nuclear
Weapons Production. Apex Press, New York. pg. 45, 67.
International Physicians for the Prevention of Nuclear
War (IPPNW) and Institute for Energy and Environmental Research (IEER).
(1992). Plutonium: deadly gold of the nuclear age. International
Physicians Press, Cambridge, Massachusetts.
Kouts, Herbert J. C. and DiNunno, Joseph J. (October
6, 1995). Safety
management and conduct of operations at the Department of Energy's defense
nuclear facilities. DNFSB/TECH-6. Defense Nuclear Facilities Safety
Board, Washington, D.C.
Leskov, S. (June 1993). Nuclear dumping: lies and incompetence.
Bulletin
of the Atomic Scientists. pg. 13.
Makhijani, A. and Makhijani, A. (January, 1995). Fissile
materials in a glass, darkly: technical and policy aspects of the disposition
of plutonium and highly enriched uranium. Institute for Energy and
Environmental Research, Takoma Park, Maryland.
Makhijani, A. (1996). Heading off the plutonium
peril. Institute for Energy and Environmental Research (IEER).
-
This IEER editorial first appeared in the Washington Post on December
5, 1996, and is an excellent thumbnail sketch of the recent decision of
the DOE to dispose of some of its excess weapons grade plutonium by incorporating
it into reactor fuel by mixing it with uranium oxide creating a mixed oxide
or MOX fuel. This editorial may be downloaded electronically from the IEER
site, see RAD 13: RADLINKS, Part II-A.
Makhijani, A. (February, 1997). Technical aspects of the
use of weapons plutonium as a reactor fuel. Science for Democratic Action.
An IEER (Institute for Energy and Environmental Research) publication.
5(4). p. 1-7.
-
This report includes information on light water reactor safety issues
as well as plutonium in spent fuel in reactors using MOX fuel.
-
"MOX spent fuel would still contain from 40 percent to over 70 percent
of the plutonium concentration in the fresh MOX fuel." (pg. 3).
Ministry of Agriculture, Fisheries and Food. (1996). Radioactivity
in food and the environment, 1995. RIFE-1. MAFF, London.
Ministry of Agriculture, Fisheries and Food and Scottish
Environment Protection Agency. (1997). Radioactivity in food and the
environment, 1996. RIFE-2. MAFF and SEPA, London.
Ministry of Agriculture, Fisheries and Food and Scottish
Environment Protection Agency. (September 1998). Radioactivity in food
and the environment, 1997. RIFE-3. Centre for Environment, Fisheries
and Aquaculture Science, MAFF and SEPA, London.
-
Annotations of this report can be found in RAD 6: Radiation Protection
Guidelines: 3. Radiological Monitoring Programs and Remediation Guides:
B. Programs Outside the USA.
National Academy of Sciences. (1971). Radioactivity
in the marine environment. Panel on Radioactivity in the Marine Environment,
National Academy of Sciences, New York.
-
A comprehensive early study of contamination of the marine
environment.
-
This report is frequently cited in this section of RADNET.
OECD, NRC and IAEA. (April, 1996). Future financial
liabilities of nuclear activities. 66-96-05-1. ISBN 92-64-14795-0.
Organization for Economic Cooperation and Development, Paris. pp. 103.
Saleska, S. et. al. (1989). Nuclear legacy: an overview
of the places, politics, and problems of radioactive waste in the United
States. Public Citizen, Washington, D.C.
U. S. Congress, OTA (Office of Technology Assessment).
(September, 1993). Dismantling the bomb and managing nuclear materials.
OTA-O-572. U.S. Government Printing Office, Washington, D.C.
U. S. Department of Energy. (September, 1988). Environmental
survey: preliminary summary report of the defense production facilities.
DOE/EH-0072. U. S. DOE, Washington, D.C.
U. S. Department of Energy. (1991). Final report
on DOE nuclear facilities. Advisory Committee on Nuclear Facility Safety
to the U.S. DOE, Washington, D.C.
3. NUCLEAR WEAPONS TEST EXPLOSIONS |
-
See Section 8 of RADNET for more
data on weapons tests fallout.
-
See Section 9 for an introduction
to the impact of weapons testing on the dietary intake of radiocesium,
etc. prior to Chernobyl.
-
See Part 6 of
this section of RADNET on Russian military source points for comments on
Russian test explosions.
-
This section of RADNET will be gradually updated and expanded.
A question for readers pursuing this section of RADNET:
Asker Aarkrog of the Riso National Laboratory in Denmark,
in his 1988 comparison of Chernobyl debris with nuclear weapons fallout
(Aarkrog, 1988, JER, p. 151-162) notes that 740 PBq of 137Cs
was released to the northern hemisphere from 423 atmospheric nuclear test
explosions. In another Riso National Laboratory publication, (Aarkrog,
1993, "Sources to Environmental Contamination in the former USSR", p. 37;
annotated in part 8 of this section) Aarkrog estimates that the 87 nuclear
explosions detonated at Novaya Zemlya alone released 370 PBq
90Sr
and 560 PBq 137Cs. Did the other 336 test explosions only release
an additional 180 PBq of 137Cs?
Aarkrog also makes the following observations: "The
integrated deposition density in the 50 to 60 N latitude band is 2.9 kBq
90Sr
m-2. (UNSCEAR,1982) In 1990, the cumulative deposit had decayed to 1.5
kBq 90Sr m-2. The corresponding level of 137Cs fallout
is a factor of 1.6 times higher, i.e. 2.4 kBq m-2 at present... the cumulative
deposit of 239,240Pu is 52 Bq m-2." (Aarkrog, et al. 1992, p.
70)
Aarkrog, A. (1990). Source terms and inventories
of anthropogenic nuclides. Report No. DK-4000. Riso National Laboratory,
Roskilde, Denmark.
Nuclear Weapons Testing Fission Yield and Waste Production:
Nuclide |
Half-life |
Representative fission yield (%) |
Normalized production (PBq per Mt fission energy) |
Sr-89 |
50.5 d |
2.56 |
590 |
Sr-90 |
28.6 a |
3.50 |
3.9 |
Zr-95 |
64.0 d |
5.07 |
920 |
Ru-103 |
39.4 d |
5.20 |
1500 |
Ru-106 |
368 d |
2.44 |
78 |
I-131 |
8.04 d |
2.90 |
4200 |
Cs-136 |
13.2 d |
0.036 |
32 |
Cs-137 |
30.2 a |
5.57 |
5.9 |
Ba-140 |
12.8 d |
5.18 |
4700 |
Ce-141 |
32.5 d |
4.58 |
1600 |
Ce-144 |
284 d |
4.69 |
190 |
Bernstein, A. and Gronlund, Lisbeth. (November 8, 1996).
Comments
by the Union of Concerned Scientists on the DOE Draft Nonproliferation
and Arms Control Assessment of Weapons-Usable Fissile Material Storage
and Disposition Alternatives and Letter from the SEAB Task Force. Union
of Concerned Scientists, Cambridge, MA.
-
This report includes extensive "...comments both on aspects of the disposition
campaign that are independent of the disposition method chosen, and on
the various disposition options under consideration." (pg. 1).
-
"...the scale of the current disposition campaign means this campaign
will fail to meet its stated goals of helping to ensure that arms reductions
are difficult to reverse and demonstrating a US commitment to irreversible
reductions." (pg. 1).
-
"...it is essential to apply permanent international IAEA safeguards
as early as possible in the disposition process. ...the near-term security
of stored plutonium and other fissile material in the US and former Soviet
Union is an 'overriding priority' (p.143 [see citation of the DOE
draft below]); indeed, an effective disposition campaign is impossible
without close attention to the near-term security of fissile material."
(pg. 1).
Bowen, V.T., Noshkin, V.E., Livingston, H.D. and Volchok,
H.L. (1980). Fallout radionuclides in the Pacific Ocean: Vertical and horizontal
distributions, largely from GEOSECS stations. Earth and Planetary Science
Letters. 49. pg. 411-434.
1973-74 |
N. Pacific |
Mean concentration in seawater |
239Pu |
0.68 d.p.m./100kg s.w. |
1978 |
N. Pacific |
Mean concentration in seawater |
239Pu |
0.13 d.p.m./100kg s.w. |
1973-74 |
N. Pacific |
Mean concentration in seawater |
137Cs |
55.6 d.p.m./100kg s.w. |
1978 |
N. Pacific |
Mean concentration in seawater |
137Cs |
44.6 d.p.m./100kg s.w. |
-
Pre-Chernobyl baseline data.
Farber, S.A. and Hodgon, A.D. (1991). Cesium-137 in
wood ash: Results of a national study. Yankee Atomic Electric Company,
Bolton, Massachusetts.
-
This report documents the presence of radiocesium in New
England hardwood ash with peak values to 21,100 pCi/kg in contrast to concentrations
in wood ash from Pacific coastal environments, which are less than 500
pCi/kg.
-
The source of these elevated concentrations in New England
wood ash is probably nuclear weapons testing fallout; there is insufficient
data to determine if Chernobyl derived radiocesium plays a role in any
of these elevated concentrations.
-
The excessive levels of radiocesium in New England wood
ash are significant enough to warrant a warning that no wood ash be recycled
as garden compost, whereby the radiocesium would become available for uptake
by root crops.
-
RADNET is soliciting any reader contributions with additional
citations on this subject.
Farrington, J.W., Goldberg, E.D., Riseborough, R.W., Martin,
J.H. and Bowen, V.T. (1983). U.S. "Mussel Watch" 1976-1978: An overview
of the trace-metal, DDE, PCB, hydrocarbon and artificial radionuclide data.
Environ.
Sci. Technol. 17. pg. 490-496.
-
A landmark article in the literature on chemical fallout,
the mussel watch has been in essence discontinued due to budgetary considerations.
-
"Elevated...239,240Pu concentrations in bivalves
from the central California coast are apparently related to enrichments
of nuclear weapons testing fallout 239,240Pu in intermediate
depth water of the North Pacific and upwelling of this water associated
with the California Current system." (pg. 490).
Fradkin, P. (1989). Fallout: an American nuclear tragedy.
University of Arizona Press, Tucson.
Hardy, E.P. Jr. (May 1, 1981). Environmental Measurements
Laboratory: Environmental report. Department of Energy, New York, N.Y.
-
1997 DOE WWW printout gives the following description
of the goals of the Environmental Measurements Laboratory (EML), which
includes 115 sampling sites operated and maintained as part of ENL's global
sampling network: "The objective of the research performed in this program
area is to provide fundamental data on natural and anthropogenic radionuclides
deposited on the earth's surface, which can be used to characterize, quantify,
and model environmental pathways, and to evaluate the environmental and
human health impacts on regional and global scales. As part of this program
a rapid response capability is maintained to support Department of Energy
(DOE) activities in radiation emergencies that arise within the U.S., and
for assessing releases that are international is scope." Information on
EML can be accessed at www.eml.doe.gov/errprog.htm or visit RAD 13: 2-D.
-
This 670 page report is one of a long series of quarterly
reports produced by the Environmental Measurements Laboratory, which began
issuing reports in 1958 as the Health and Safety Laboratory and continues
to issue reports today. The very first report was HASL-42 Environmental
Contamination from Weapons Tests; all EML reports may be accessed and purchased
from the National Technical Information Service; the EML WWW site contains
a complete list (126 pages) of all the publications and reports ever issued
by this laboratory, and not much else. URL: http://www.eml.doe.gov/PUBS/PUBCROSS.HTM
-
The forte of EML is its extensive documentation of weapons
testing derived 90Sr; thousands of pages of documents and hundreds
of reports have been devoted to this specific radionuclide. Another EML
forte is stratospheric inventories of 90Sr, 95Zr,
238Pu,
and 239Pu as well as 137Ce and
144Ce.
An update of stratospheric nuclide inventories to July 1979 is contained
in this report in Vol. I, page 341. For example, the Nov. 17, 1976 Chinese
atmospheric nuclear test resulted in the following stratospheric inventories
of 90Sr: Oct. 1978: 45 kCi; Apr. 1979: 34 kCi; July 1979: 19
kCi. The 137Cs / 90Sr inventory ratio is noted as
1.6 +/-.2 for the years 1970-79 (page I-343).
-
This report provides a number of interesting tables pertaining
to weapons tests (page I-19 to I-25):
-
Table 1-A: Date and yields of nuclear detonations of the
People's republic of China: max. yield 4,000 KT, 11/17/76.
-
Table 1-B: Dates and yields of nuclear detonations by
the Republic of France: max. yield 1,000 KT, 08/14/71.
-
Table 2: Movement of radioactive debris from atmospheric
tests: max. movement time 21 days: Eniwetok Atoll to Debracken, Hungary;
debris travel time from Siberia to Washington, DC, 16 days; from Bikini
Island to Rio de Janeiro, 21 days; Nevada Test Site to Ottawa, Canada,
1 to 2 days; Nevada Test Site to Frieburg, W. Germany, 7 days.
-
Table 3: Travel time of radioactive debris from Chinese
tests to various sites: max. transport time was 40 to 47 days to Chilton,
UK; most transport times were 2 weeks or less.
-
Table 4: Movement of radioactive debris from underground
tests: transport times for leaky Nevada Test Site to European locations
were 8 - 15 days.
-
Table 5: Maximum gross beta activity observed after the
first French test of Sahara on 13/2/60: Tamale, Ghana surface air contamination:
1,000 pCi/m3; Aix la Chappelle, W. Germany rain water contamination:
14,000 pCi/liter; Bombay, India ground deposition: 169 MC/KM2.
- Note that EML is now (as of 2009) called the National Urban Security Technology Laboratory (NUSTL). There are links online to the older reports at http://www.wipp.energy.gov/namp/emllegacy/publications.htm.
International Atomic Energy Agency. (1998). The radiological
situation at the atolls of Mururoa and Fangataufa: Reports by an International
Advisory Committee: Radiological Assessment Reports Series. STI/PUB/1028/ES.
IAEA, Austria.
International Physicians for the Prevention of Nuclear
War (IPPNW). (September, 1992). Nuclear test tally 1992. Vital Signs.
IPPNW, Cambridge, Massachusetts. 5(3) pg. 4.
International Physicians for the Prevention of Nuclear
War (IPPNW) and Institute for Energy and Environmental Research (IEER).
(1991). Radioactive heaven and earth: the health and environmental effects
of nuclear weapons testing in, on, and above the earth. The Apex Press,
New York.
Livingston, H.D. and Bowen, V.T. (1979). Pu and 137Cs
in coastal sediments. Earth and Planetary Science Letters, 43,
29-45.
1973 |
Buzzard Bay |
0-2 cm Sediment core |
239,240Pu |
160 d.p.m./kg dry sediment |
-
Peak concentration of fallout 239,240Pu in
sediment to 2.5 mCi/km2
Machta, L. and Telegada, K. (1970). Radioiodine levels
in the U.S. public health service pasteurized milk network from 1963-1968
and their relationship to possible sources. Health Physics. 19,
pg. 469-485.
April 14, 1965 |
Palanquin, NV |
Milk |
131I |
11,000 pCi/l |
April 23, 1963 |
Pin stripe, NV |
Milk |
131I |
4,800 pCi/l |
-
One of the rare citations with media specific data on
close-in local weapons testing fallout.
-
Also see Section 8, Baseline Data, and Section 9, Dietary
Intake, for more data on nuclear weapons testing contamination.
Makhijani, A., Hu, H. and Yih, K. (1995). Nuclear wastelands:
A global guide to nuclear weapons production and its health and environmental
effects. Massachusetts Institute of Technology, Boston, MA.
-
A comprehensive general summary of nuclear weapons production
facilities and an overview of the principal health physics and environmental
issues associated with each site.
-
This publication acknowledges the lack of documentation
necessary for comprehensive evaluation of the health and environmental
effects of these weapon production sites: "One legacy of the long history
of nuclear weapons production in the United States is a large number of
'formerly used sites that had been contaminated and abandoned or restored
to civilian use without appropriate cleanup. There is evidence of a similar
picture in Russia.' " (p. 63). "Neither the AEC nor DOE monitored many
sources of radioactive emissions, including sources that generated considerable
amounts of radioactive waste." (pg. 185).
-
Table 6.2, pages 189-200 provides a partial list of locations
with nuclear weapons related activities (and therefore contamination),
but does not include all the sites now undergoing DOE environmental remediation
efforts as listed in DOE publications.
-
This publication provides a comprehensive listing of the
types of contamination originating at U. S. and well as foreign weapons
production facilities (radioactive, chemical and heavy metals contamination)
but provides very little data on the actual amounts of the contamination.
-
Table 6.10 reprints high-level waste inventories at 3
U. S. facilities as provided by the U. S. DOE integrated database discussed
in this section of RADNET. The authors of this publication make no comments
or observations about the fact that the 970 million curies of military
high-level waste cited in this table are an inadequate accounting of total
U. S. military high-level waste production or that there may be other locations
having contained or uncontained inventories of high-level waste other than
Hanford, Savannah River or the Idaho National Laboratory. Table 6.10 omits
the DOE listing for West Valley New York.
-
This text is particularly useful in its focus on the lack
of data for evaluating worker exposure to contamination.
-
This publication contains an excellent summary of Russian
and British weapons production contamination source points. Table 11.1,
page 533-553 is an overview of nuclear weapons related activities throughout
the world other than U. S. locations. Table 12.1, page 581, contains nuclear
weapons materials inventories for countries with nuclear weapons capabilities.
-
This is the most comprehensive guide to world wide nuclear
weapons production presently available despite its paucity of data pertaining
to actual inventories of contained as well as uncontained high-level waste.
Miller, Pam. Return to Amchitka -- A Greenpeace Report.
1436 U Street, NW, Washington, DC.
-
Amchitka Island was the site of three underground nuclear
tests (1965, 1969, 1971), the latter of which (Cannikin, 5 megatons) was
the largest underground nuclear test in US history. This test was also
the seminal event which stimulated the organization of the environmental
group Greenpeace which evolved from the 1971 protest of this test.
-
Greenpeace returned to this island in the Bering Sea to
check on possible venting of contamination from this site and documented
contamination in moss and algae samples including Cs-137 (p.v.: 9.96 pCi/g(ash)),
Pu-239/240 (p.v.: .15 pCi/g(ash)) and Am-241 (p.v.: .094 pCi/g(ash)).
-
While there is not enough data or control samples to determine
how much cesium and plutonium result from stratospheric fallout versus
these three underground tests, the presence of americium 241(a constituent
of weapons testing emissions as well as the daughter product of plutonium
241) indicates, according to Greenpeace, that leakage is occurring from
this underground test which was made too close to the surface.
-
A copy of this report may be obtained from Greenpeace:
see RADNET section 13: RADLINKS Part 2-B. Also see the americium-241 alert
in RADNET Section 15.
Momoshima, N. and Takashima, Y. (1986). Radionuclide concentrations
in several seaweeds and their annual variations. Journal of Radioanalytical
and Nuclear Chemistry. 99(2). pg. 367-377.
-
"A marked change was observed in the number of radionuclides
in seaweeds. The increase of radionuclides is attributed to contamination
by radioactive fallout from Chinese nuclear explosion tests." (pg. 367).
National Cancer Institute.
(August 1, 1997). Estimated exposures and thyroid doses received by
the American people from Iodine-131 in fallout following Nevada atmospheric
nuclear bomb tests. NCI, National Institute of Health, Washington,
D.C.
-
The full report including a color coded map detailing county-by-county
exposure estimates is available on the Internet at URL: http://rex.nci.nih.gov/massmedia/Fallout/index.html.
-
For an additional critique of the NCI report by IEER (Institute for
Energy and Environmental Research) go to URL: http://www.ieer.org/ieer/latest/iodnart.html.
-
Hard copy is available from the National Cancer Institute, Office of
Cancer Communications, Building 31, Room 10A24, Bethesda, MD 20892. It
is 100,000+ pages.
-
"The National Cancer Institute (NCI) report contains an assessment of
radioactive Iodine-131 (I-131) fallout exposure from the nuclear bomb tests
that were carried out at the Nevada Test Site in the 1950s and 1960s. In
1982, Congress passed legislation calling for the Department of Health
and Human Services to develop methods to estimate I-131 exposure to the
American people, to assess thyroid doses from I-131 received by individuals
across the country from the Nevada tests, and to assess risks for thyroid
cancer from these exposures. The fallout report fulfills the first two
of these three requirements." (Backgrounder Questions and Answers).
-
"The report includes county-by-county estimates of average I-131 doses
to the thyroid for persons living or born in the contiguous 48 states during
the period when the bomb tests were carried out, mostly in the 1950s."
(Backgrounder Questions and Answers).
-
"The report shows that everyone living in the contiguous 48 states was
exposed to I-131 at some level. The average cumulative thyroid dose to
the approximately 160 million people in the country at the time was about
2 rads." (Backgrounder Questions and Answers).
-
"Meteorological modeling and the re-analysis of historical monitoring
data are the two methods used to estimate the amounts of 131I
that were deposited on the ground following each test. For both approaches,
the assumption is made that all of the 131I released to the
atmosphere was in particulate form, as were the majority of radionuclides
produced in the atmospheric nuclear weapons tests." (Technical Summary).
-
"The radioactive cloud that was formed after an atmospheric detonation
near the ground surface usually was in the shape of a mushroom, extending
from the ground surface to the highest layers of the troposphere, and occasionally
reaching into the stratosphere. It contained hundreds of different radionuclides,
including 131I. ... The 131I activity per unit yield
was found to be about 150 kCi kt-1 of fission for the tests considered
in this report and the total activity of 131I released into
the atmosphere was estimated to be about 150 MCi. (Technical Summary).
-
"Deposition of 131I on the ground results from two processes:
the impaction of aerosols on the ground surface (dry deposition) and precipitation
(wet deposition). In the western part of the country, most of the deposition
of 131I was due to dry processes ... [in contrast to the eastern
part of the country] where most of the 131I deposition occurred
as a result of precipitation." (Technical Summary).
-
The NCI report is significant in that it reveals AEC - DOE monitoring
data which clearly documented much greater dispersion of weapons testing
fallout than the government admitted at the time of the tests.
-
Also see our special appendix: Contaminated
milk: A paradigm and WHO's 1986, post-Chernobyl
national safety guidelines for 131I in milk
Norris, R.S. and Arkin, W.M. (May 1992). Nuclear notebook:
Proposed U.S. and C.I.S. strategic forces. The Bulletin of the Atomic
Scientists. pg. 48-49.
Noshkin, V.E. (1972). Ecological aspects of plutonium
dissemination in aquatic environments. Health Physics, 22,
537-549.
1964 |
Bikini |
Snapper (live) |
239Pu |
7000 pCi//kg wet |
1970 |
Cape Cod |
Striped bass (backbone) |
239Pu |
0.2 pCi/kg |
-
"...Plutonium is found widespread among planktonic, pelagic
and benthic organisms" (pg. 537).
-
"Bone and liver are major repositories for plutonium in
marine vertebrates..." (pg. 537).
-
"In marine sediments, as in soils, plutonium is more mobile
than was originally expected." (pg. 537).
-
"...It now appears that when the relative biological effectiveness
of alpha vs. gamma or beta radiation is considered, fallout
239Pu
contributes more than fallout 90Sr or 137Cs to the
artificial radiation exposure of many marine species." (pg. 537).
-
Excellent bibliography. A landmark article in ancient
hard copy.
Roos, P., Holm, E., Persson, R.B.R., Aarkrog, A. and Nielsen,
S.P. (1994). Deposition of 210Pb, 137Cs,
239+240Pu,238Pu
and 241Am in the Antarctic Peninsula area.
J. Environ. Radioactivity.
24(3). pg. 235-252.
1989 |
Livingstone Island |
Grass and soil |
137Cs |
392 Bq/m2 |
1989 |
Livingstone Island |
Lichen |
239Pu |
11.60 Bq/m2 |
-
137Cs to 20 Bq/kg (544 pCi/kg) in dry sediment.
United States Department of Energy. (1994). United
States nuclear weapons tests, July 1945 through December 1992. Report
No. DOE/NV-209, Rev. 14. U.S. Department of Energy, Washington, D.C.
-
A detailed listing of all U.S. Nuclear weapons tests.
United States Department of Energy.
(October 1, 1996). Draft nonproliferation and arms control assessment
of weapons-usable fissile material storage and plutonium disposition alternatives.
U.S. Department of Energy, Washington, D.C.
United States Department of Energy. (February 1998).
Accelerating
cleanup: Paths to closure. DOE/EM-0342. Office of Environmental
Management, U.S. DOE, Washington, DC.
Venter, A. J. (March 31, 1999). New generation of nuclear
weapons from radioactive waste. Jane's Defence Weekly. 31(13).
-
"There is a strong feeling within the nuclear establishment that both
America and France have actually conducted nuclear explosive experiments
with neptunium 237, thus proving the suitability of this material for use
in nuclear explosives" (David Albright, head of the Institute for Science
and International Security).
-
"Said Albright, 'the world inventory of neptunium and americium is estimated
to exceed 80 metric tonnes, or enough for more than 2,000 nuclear warheads.'
He told JDW that the amount is growing by about 10 tonnes a year."
An entire issue of Health Physics (vol. 72 no. 7, July
1997) has been devoted to the history of atomic weapons testing in the
Marshall Islands, which include the Bikini Test Site, Enewetak Atoll, and
other northern Marshall Islands atolls. Testing began in 1946 and lasted
until 1958. Topics include the history of weapons testing, radiological
monitoring, dose assessment, health effects and environmental studies at
these test sites. Several of the contributed papers are cited below. Abstracts
of all the papers in this and other Health Physics issues can be downloaded
from http://www.wwilkins.com/.
Donaldson, Lauren R., Seymour, Allyn H. and Nevissi,
Ahmad E. (July 1997). University of Washington's radioecological studies
in the Marshall Islands, 1946-1977. Health Physics. 72(7).
Eisenbud, Merril. (July 1997). Monitoring distant fallout:
The role of the Atomic Energy Commission Health and Safety Laboratory during
the Pacific tests, with special attention to the events following BRAVO.
Health
Physics. 72(7).
Niedenthal, Jack. (July 1997). A history of the people
of Bikini following nuclear weapons testing in the Marshall Islands: With
recollections and views of elders of Bikini Atoll. Health Physics.
72(7).
Noshkin, V.E., et. al. (July 1997). Past and present
levels of some radionuclides in fish from Bikini and Enewetak Atolls. Health
Physics. 72(7).
Noshkin, V.E. and Robison, W.L. (July 1997). Assessment
of a radioactive waste disposal site at Enewetak Atoll. Health Physics.
72(7).
Robison, W.L., et. al. (July 1997). The northern Marshall
Islands radiological survey: Data and dose assessments. Health Physics.
72(7).
Simon, Steven, L. (July 1997). A brief history of people
and events related to atomic weapons testing in the Marshall Islands. Health
Physics. 72(7).
Simon, Steven L. and Graham, J.C. (July 1997). Findings
of the first comprehensive radiological monitoring program of the Republic
of the Marshall Islands. Health Physics. 72(7).
United States Energy Research and Development. (1975).
Preliminary
external-dose estimates for future Bikini Atoll inhabitants. Preliminary
report No. UCRL-51879. USERD.
Johnston Atoll consists of four islands 825 miles southwest
of Hawaii. Currently, it is managed by the U.S. Department of Fish
and Wildlife Services as a National Wildlife Refuge. It has been
used by the military since the mid-1930's, and was the site of several
air atomic tests during the early 1960's. It is the site of JACADS
(Johnston Atoll Chemical Agent Disposal System) for the destruction of
chemical weapons. JACADS is run by the U.S. Army's Chemical Stockpile
Disposal Project, and expects its stockpile of chemical weapons to all
be destroyed by 2000.
Field, Michael. (March 18, 1999). Lonely Pacific atolls
deadly weapons nearly gone but leakages remain. Agence France Presse.
-
"The clean up has included scattered plutonium. A nuclear missile
failed to lift-off from the Johnston pad and exploded. The plutonium
core did not go critical but was scattered along a thousand metre (yard)
length of shoreline."
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