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4. CHERNOBYL PLUME:
COUNTRY-BY-COUNTRY SUMMARY (I - R) |
(The listing is alphabetical: A-H, Italy,
Japan,
Monaco,
Netherlands,
Norway,
Poland,
Portugal,
Russia
and former USSR,
S-Z; the U.S.A.
follows all the others)
The following section of our website has been translated
into Italian
by Humus - Progetto.
(The Humus Project: The effects of Chernobyl contamination on the
soil.)
Astori, E. et. al. (April 1, 1999). Surface contamination
of radiocesium measured and calculated in South Piemonte (Italy). J.
Environ. Radioactivity. 45(1). pg. 29-38.
Baldini, E., Bettoli, M.B. and Tubertini, O. (1987).
Measurements on Chernobyl fallout in forest vegetation. Inorganica Chimica
Acta. 140. pg. 331-333.
July 10, 1986 |
N. Italy |
Lichens |
137Cs |
12,100 Bq/kg |
July 10, 1986 |
N. Italy |
Spruce twigs |
137Cs |
3,750 Bq/kg |
July 10, 1986 |
N. Italy |
Scotch pine twigs |
137Cs |
2,520 Bq/kg |
July 10, 1986 |
N. Italy |
Larch twigs |
137Cs |
1,600 Bq/kg |
-
Lesser amounts of 141Ce, 144Ce and
140Ba-140La
were noted.
Battiston, G.A., Degetto, S., Gerbasi, R., Sbrignadello,
G. and Tositti, L. (1987). The deposition of Chernobyl fallout in north-east
Italy. Inorganica Chimica Acta. 140. pg. 327-329.
May 1, 1986 |
Padua |
Air concentration, average values |
131I |
15,577 mBq/m3 |
May 1, 1986 |
Padua |
Air concentration, av |
132I (132Te) |
10,550 mBq/m3 |
May 1, 1986 |
Padua |
Air concentration, av |
103Ru |
4,070 mBq/m3 |
May 1, 1986 |
Padua |
Air concentration, av |
134,137Cs |
2,712 mBq/m3 |
-
"137Cs deposition in N. Italy ranged from 60,000
Bq/m2 down to 2,000-5,000 Bq/m2 on the coastal plain."
(pg. 329).
-
15,577 millibecquerels (mBq) equals 15,577,000 microbecquerels
(µBq).
Battiston, G.A., Degetto, S., Gerbasi, R., Sbrignadello,
G. and Tositti, L. (1988). Fallout distribution in Padua and northeast
Italy after the Chernobyl nuclear reactor accident. J. Environ. Radioactivity.
8. pg. 183-191.
30 April 1986 |
NE Italy |
Air |
131I |
28.6 Bq/m3 |
30 April 1986 |
NE Italy |
Air |
132Te |
19.2 Bq/m3 |
May 1986 |
Padua |
Soil |
137Cs |
45,000 Bq/m2 |
-
28.6 becquerels (Bq) equals 28,600,000 microbecquerels
(µBq).
-
Average cumulative deposit from weapons test fallout from
239Pu
noted as 62 Bq/m2.
Battiston, G.A., Degetto, S., Gerbasi, R. and Sbrignadello,
G. (1989). Radioactivity in mushrooms in northeast Italy following the
Chernobyl accident. J. Environ. Radioactivity. 9. pg. 53-60.
-
Peak concentration of 137Cs in edible mushrooms
noted as 27,626 Bq/kg of which 21,978 Bq were Chernobyl-derived.
-
Total 134,137Cs deposition to 60,000 Bq/m2
and higher (1:2 initial isotope ratio).
Boccolini, A., Gentili, A., Guidi, P., Sabbatini, V. and
Toso, A. (1988). Short communication: Observation of silver 110m in the
marine mollusc Pinna nobilis. J. Environ. Radioactivity.
6. pg. 191-193.
-
High activity ratios of 110mAg to 137Cs
in the marine mollusk Pinna nobilis were recorded in the range of
15-36 Bq/kg, compared to that in dust in air filters, 0.4-0.5, illustrating
the tendency of this very large bivalve mollusk to concentrate 110mAg
present in seawater.
Bonnazzola, G.C., et. al. (1993). Profiles and downward
migration of 137Cs and 106Ru deposited on Italian
soils after the Chernobyl accident. Health Physics. 64(5). pg. 479-484.
Capra, E., Drigo, A. and Menin, A. (1989). Cesium-137
urinary excretion by northeastern (Pordenone) Italian people following
the Chernobyl nuclear accident. Health Physics. 57(1). pg. 99-106.
May 20, 1986 |
Pordenone |
Milk |
137Cs |
254 Bq/dm3 |
Sept 30, 1987 |
Pordenone |
Meat |
137Cs |
395 Bq/kg |
-
Peak urinary excretion of 137Cs occurred 300
to 425 days after main fallout cloud passage on May 5, 1986: pv 15-20 Bq/day.
Gentili, A., Gremigni, G. and Sabbatini, V. (1991). Ag-110m
in fungi in central Italy after the Chernobyl accident. J. Environ.
Radioactivity. 13(1). pg. 75-78.
-
110Ag activity in fungi collected in autumn
1986 was not detectable.
-
"Samples collected in 1988 and 1989 showed a remarkable
accumulation of 110mAg (to 28 Bq/kg on Dec. 16, 1988)." (pg.
75).
-
"110mAg was indeed present in soils in 1986
but that it was not available to fungi because of its chemical form and
because of lack of rainfall." (pg. 75).
Lofti, M., Notaro, M., Piermattei, S., Tommasino, L. and
Azimi-Garakani, D. (1990). Radiocesium contents of meat in Italy after
the Chernobyl accident and their changes during the cooking process. J.
Environ. Radioactivity. 12(2). pg. 179-184.
-
Radiocesium content of lamb is higher than any other meats
considered. (pg. 179).
-
"When meat is cooked in salt water (14%), the activity
decreases by as much as 80%." (pg. 179).
Orlando, P., Gallelli, G., Perdelli, F. DeFlora, S. and
Malcontenti, R. (1986). Alimentary restrictions and 131I in
human thyroids. Nature. 324. pg. 23.
May 3- June 16, 1986 |
Genoa, Italy |
51 adults, thyroid |
131I |
6.5 Bq/g, average |
May 11, 1986 |
Genoa, Italy |
Milk |
131I |
135,000 Bq/kg |
-
The average weight of a thyroid is 20 grams.
Roca, V., Napolitano, Speranza, P.R. and Gialanella, G.
(1989). Analysis of radioactivity levels in soils and crops from the Campania
region (south Italy) after the Chernobyl accident. J. Environ. Radioactivity.
9. pg. 117-129.
20 May - 5 June 1986 |
S. Italy |
Green wheat |
137Cs |
800 Bq/kg |
June-Oct. 1986 |
S. Italy |
Ground deposition |
137Cs |
8,100 Bq/m2 |
June-Oct. 1986 |
S. Italy |
Ground deposition |
103Ru |
11,900 Bq/m2 |
Spezzano, P., Bortoluzzi, S., Giacomelli, R. and Massironi,
L. (1994). Seasonal variations of 137Cs activities in the Dora
Baltea River (Northwest Italy) after the Chernobyl accident. J. Environ.
Radioactivity. 22(1). pg. 77-88.
-
"Increased water concentrations of 137Cs in
summer were attributed to cesium deposition and accumulation on snow covered
surfaces in winter and a delayed release in summer during ice and snow
melting." (pg. 77).
Spezzano, P. and Giacomelli, R. (1991). Transport of
131I
and 137Cs from air to cows' milk produced in north-western Italian
farms following the Chernobyl accident. J. Environ. Radioactivity.
13(3). pg. 235-250.
-
"Predicted values were 2.6, 2.1, and 5.6 times higher
than observed results for 131I, and 4.3, 3.7 and 16 times higher
for 137Cs, for vegetation to air, milk to vegetation, and milk
to air ratios, respectively." ( pg. 235).
Spezzano, P. and Giacomelli, R. (1990). Radionuclide concentrations
in air and their deposition at Saluggia (northwest Italy) following the
Chernobyl nuclear accident. J. Environ. Radioactivity. 12(1). pg.
79-92.
30 Apr-May 8 |
Saluggia |
Ground deposition |
137Cs |
11,000 Bq/m2 |
May 2 |
Saluggia |
Air concentration |
131I |
8,510 Bq/m3 |
-
"97% of the total deposition occurred between April 30
and May 7." (pg. 89).
-
"Wet deposition... was the dominant process in controlling
deposition to the ground for the particulate radionuclides." (pg. 89).
Aoyama, M., Hirose, K. and Sugimura, Y. (1991). The
temporal variation of stratospheric fallout derived from the Chernobyl
accident. J. Environ. Radioactivity. 13(2). pg. 103-116.
-
Chernobyl-derived stratospheric fallout continued until
the end of 1988.
-
Annual 137Cs deposits were 135, 0.95, and 0.57
Bq/m2, with 80% of this from Chernobyl.
-
Peak weapons fallout of 137Cs was in June 1963
at Tokyo: 548 Bq/m2.
-
Resuspension of 137Cs contributed 2% and 34%
to the annual deposition in 1987 and 1988 respectively. (pg. 113).
Aoyama, M., Hirose, K. and Sugimura, Y. (1987). Deposition
of gamma-emitting nuclides in Japan after the reactor-IV accident at Chernobyl.
Journal
of Radioanalytical and Nuclear Chemistry, Articles. 116(2).
pg. 291-306.
May, 1986 |
Akita |
30 day cumulative deposition |
131I |
18,792 Bq/m2 |
May, 1986 |
Akita |
30 day cumulative deposition |
137Cs |
414 Bq/m2 |
May, 1986 |
Akita |
30 day cumulative deposition |
103Ru |
1,098 Bq/m2 |
Aoyama, M., Hirose, K., Suzuki, Y., Inoue, H. and Sugimura,
Y. (1986). High levels of radioactive nuclides in Japan in May. Nature.
321. pg. 819-820.
-
The Chernobyl plume arrived in Japan in the form of an
abrupt change of atmospheric radioactivity - with an increase of about
a thousand fold in air concentration of 137Cs.
Higuchi, H., Fukatsu, H., Hashimoto, T., Nonaka, N., Yoshimizu,
K., Omine, M., Takano, N. and Abe, T. (1988). Radioactivity in surface
air and precipitation in Japan after the Chernobyl accident.
J. Environ.
Radioactivity. 6. pg. 131-144.
-
Twenty nuclides were observed in two kinds of plumes in
early (1,500 m) and late May (6,300 m), with a highest level in Northwestern
Japan; the average deposition of 137Cs from May 1 to May 22
was 95 Bq/m2, 550 times higher than the
pre-Chernobyl value.
Hisamatsu, S., Takizawa, Y. and Abe, T. (1987). Reduction
of 131I content in leafy vegetables and seaweed by cooking.
J.
Radiat. Res. 28(1). pg. 135-140.
May 1986 |
Akita |
Ground deposition |
131I |
2,500 Bq/m2 |
May 1986 |
Akita |
Edible seaweed |
131I |
1,300 Bq/kg fresh weight |
-
"The decontamination ratio of 131I content
in leafy vegetables and edible wild grass samples boiled in water to that
in washed samples was 0.51 +/- 0.21. The ratio of 131I content
in leafy vegetables and edible wild grass samples boiled in water to that
in washed samples was 0.51 +/- 0.19 on an average." (pg. 135).
Imanaka, T. and Koide, H. (1986). Fallout in Japan from
Chernobyl. J. Environ. Radioactivity. 4. pg. 149-153.
-
Twenty nuclides were detected in air, the dominant species
being 131I, 103Ru, 137Cs and 134Cs;
maximum air concentration for 131I was 0.8 Bq/m3
(800,000 µBq/m3) on May 5.
Ishida, J., Miyagawa, N., Watanabe, H., Asano, T. and
Kitahara, Y. (1988). Environmental radioactivity around Tokai-Works after
the reactor accident at Chernobyl. J. Environ. Radioactivity. 7.
pg. 17-27.
May, 1986 |
Tokai-mura, Japan |
aerosol associated |
131I |
1 x 10-1 Bq/m3 |
May, 1986 |
Tokai-mura, Japan |
gaseous in air |
131I |
3 x 10-1 Bq/m3 |
May, 1986 |
Tokai-mura, Japan |
plants |
131I |
2.1 x 102 Bq/kg |
Kawamura, H., Sakurai, Y., Shiraishi, K. and Yanagisawa,
K. (1988). Concentrations of 131I in the urine of Japanese adults
and children following the Chernobyl nuclear accident. J. Environ. Radioactivity.
6. pg. 185-189.
-
131I peak concentrations to 3.3 Bq/dm3
in a male adult.
Kusakabe, M. and Ku, T.L. (1988). Chernobyl radioactivity
found in mid-water sediment interceptors in the N. Pacific and Bering Sea.
Geophysical
Research Letters. 15(1). pg. 44-47.
-
Nuclides in fine air-borne particles have been incorporated
into biogenic material formed in the surface ocean and transferred downward
with velocities of +/- 100 meters per day.
Nishizawa, K., Takata, K., Hamada, N., Ogata, Y., Kojima,
S., Yamashita, O., Ohshima, M. and Kayama, Y. (1986). 131I in
milk and rain after Chernobyl. Nature. 324. pg. 308.
-
131I concentrations in milk to 400 pCi/l, 4-5
times higher than in rainwater.
Noguchi, H. and Murata, M. (1988). Physiochemical speciation
of airborne 131I in Japan from Chernobyl. J. Environ. Radioactivity.
7. pg. 65-74.
-
"Physiochemical forms of 131I were 19% particulate
iodine, 5% I2, 6% HOI and 70% organic iodides." (pg. 65).
Ooe, H., Seki, R. and Ikeda, N. (1988). Particle-size
distribution of fission products in airborne dust collected at Tsukuba
from April to June 1986. J. Environ. Radioactivity. 6. pg. 219-223.
-
137Cs activity over a thousand times the usual
level was detected in airborne dust from the end of April to the beginning
of May. AMAD (activity median aerodynamic diameters) range were 0.25 to
0.70 µm.
Seki, R., Endo, K. and Ikeda, N. (1988). Determination
of radioiodine species in rain water collected at Tsukuba near Tokyo. J.
Environ. Radioactivity. 6. pg. 213-217.
-
Iodide was the predominant species; no iodate was noted
1-6 May; iodate concentration was 1/3 that of iodide in mid-May sampling
period; by June 1, 131I species were not detectable.
Uchiyama, M. and Kobayashi, S. (1988). Consequences of
the Chernobyl reactor accident on the 137Cs internal dose to
the Japanese population. J. Environ. Radioactivity. 8. pg. 119-127.
-
Before the Chernobyl accident 137Cs body burdens
were about 30 Bq, rising the following year, 1986, to over 50 Bq with values
still increasing in May of 1987. This compares to body burdens in England
of 250-450 Bq. Differences in 137Cs body burdens among individuals
studied have become smaller with time.
Yoshida, S., Muramatsu, Y. and Ogawa, M. (1994). Radiocesium
concentrations in mushrooms collected in Japan. J. Environ. Radioactivity.
22(2). pg. 141-154.
1990 |
Akita |
Mushrooms |
137Cs |
16,300 Bq/kg |
-
Mushroom 137Cs activity varied widely; no other
sample was greater than 3,110 Bq/kg.
-
"The proportions of 137Cs originated from the
Chernobyl accident... and were calculated in the range of 7-60% (1989)
and 10-23% (1990)" (pg. 143).
Ballestra, S.B., Holm, E., Walton, A. and Whitehead,
N.E. (1987). Fallout deposition at Monaco following the Chernobyl accident.
J.
Environ. Radioactivity. 5. pg. 391-400.
May 4-5, 1986 |
Monaco |
Deposition in rainfall |
131I |
7,517 Bq/m2 |
May 4-5, 1986 |
Monaco |
Deposition in rainfall |
103Ru |
2,350 Bq/m2 |
-
A total of 33 radioisotopes were detected; one week later,
activities had fallen to about 1% of peak values.
Fowler, S.W., Buat-Menrad, P., Yokoyama, Y., Ballestra,
S., Holm E. and van Nguyen, H. (1987). Rapid removal of Chernobyl fallout
from Mediterranean surface waters by biological activity. Nature.
329. pg. 86-88.
-
141Ce and 144Ce were rapidly removed
from surface waters and transported to 200 m in a few days primarily by
zooplankton grazing ( by rapidly sinking fecal pellets).
Whitehead, N.E., Ballestra, S., Holm, E. and Walton, A.
(1988). Air radionuclide patterns observed at Monaco from the Chernobyl
accident. J. Environ. Radioactivity. 7. pg. 249-264.
-
Two pulses of Chernobyl-derived radioactivity were noted:
the first on April 29-30; the second activity peak was May 4-5, allowing
detection and differentiation of two different phases of the accident,
even though Monaco and Chernobyl are about 1900 km apart. (pg. 260-61).
-
Unusual radionuclides such as 105Ru, 111Ag, 125Sn and
126Sb were identified as being present in small amounts, out of a total
of 34 nuclides observed.
Whitehead, N.E., Ballestra, S., Holm, E. and Huynk-Ngoc,
L. (1988). Chernobyl radionuclides in shellfish. J. Environ. Radioactivity.
7. pg. 107-121.
-
Chernobyl-derived radionuclides in mussels (Mytilus
galloprovincialis) included 129Te: 2,203 Bq/kg; 129mTe:
2,774 Bq/kg; 131I: 5,387 Bq/kg; 132Te: 3,168 Bq/kg
(all soft parts, wet weight).
-
Fifty days later, the concentration factor was 1/20 to
1/50 of the May 7 values.
Frissel, M.J., Stoutjesdijk, J.F., Koolwijk, A.C. and
Koster, H.W. (1987). The Cs-137 contamination of soils in the Netherlands
an its consequences for the contamination of crop products. Netherlands
Journal of Agricultural Science. 35. pg. 339-346.
-
Total 137Cs deposition levels in the Netherlands
in 1954 to 1982: 4,600 Bq/m2, even distribution. Remaining weapons
fallout deposition in soils in 1987, 1,500 Bq 137Cs.
-
Chernobyl-derived radiocesium deposition levels: estimated
dry deposition in May, 1986 500 Bq/m2, even distribution. Estimated
wet deposition May, 1986, 0-5,500 Bq/m2, extremely variable
distribution.
Sloof, J.E. and Wolterbeek, B.T. (1992). Lichens as biomonitors
for radiocesium following the Chernobyl accident. J. Environ. Radioactivity.
16(3). pg. 229-242.
1986 |
Netherlands |
Ground deposition |
137Cs |
6,000 Bq/m2 |
1986 |
Netherlands |
Lichen (Armelia) |
137Cs |
6,100 Bq/kg |
-
Activity concentration levels of Chernobyl-derived radiocesium
in lichens closely followed ground deposition levels in the Netherlands
(Activity per lichen dry weight vs. activity deposited per unit area (m2)
= approximately 1. (pg. 229).
van Dam, H. (1986). Silver from Chernobyl. Nature.
324. pg. 216.
-
Chernobyl-derived radiosilver probably originated from
200 in core neutron detectors which had emitters composed of silver.
Voors, P.I. and van Weers, A.W. (1991). Transfer of Chernobyl
radiocesium (134Cs and 137Cs) from grass silage to
milk in dairy cows. J. Environ. Radioactivity. 13(2). pg. 125-140.
-
1986 radiocesium contaminated grass silage was used as
feed in 1988 for dairy cows. (Average 1986 grass silage: 137Cs
171.8 Bq/kg, dry weight.) Milk: to 4.7 Bq/l.
-
40-55% of the daily radiocesium intake was excreted daily.
-
Average excretion rate of radiocesium for two cows was
4-5% in milk; 5-9% in urine and 32-43% in feces.
Online radiation fallout maps of Northern Europe: map
1 and map
2.
Blakar, I.A., Hongve, D. and Njastad, O. (1992). Chernobyl
cesium in the sediments of Lake Hoysjoen, central Norway. J. Environ.
Radioactivity. 17(1). pg. 49-58.
-
Total radiocesium activity in soils in affected areas
of Norway was in the range of 5,000-200,000 Bq m-2.
-
Study area deposition was about 50,000 Bq m-2.
-
Sediment concentration was similar to that in surrounding
soil but higher accumulation was noted in a riverine plume due to runoff
from frozen wetland after deposition and subsequent melting.
-
Lake sediment contamination range "was rather homogeneous
with activities between 25 and 75 kBq m-2 in most parts of the
lake." (pg. 53).
-
Stationary populations of brown trout and antic char contained
about 1% of activity in the sediments." (pg. 53).
Brittain, J.E., Storruste, A. and Larsen, E. (1991). Radiocesium
in brown trout (Salmo trutta) from a subalpine lake ecosystem after
the Chernobyl reactor accident. J. Environ. Radioactivity. 14(3).
pg. 181-192.
Sep. 20 |
Ovre Heimdalsvatn |
Brown trout |
134,137Cs |
12,500 Bq/kg wet weight |
Aug. 28 |
Ovre Heimdalsvatn |
Lichen |
134,137Cs |
60,000 Bq/kg wet weight |
-
1986 average total cesium content rose to 7000 Bq/kg wet
weight, falling to 4,000 Bq in 1988. No further declines were noted in
1988 and 1989, though there was considerable variation in content measured
in individual fish.
-
An observed half life of 3.0 years for 137Cs
in trout was estimated.
Hongve, D., Blakar, I.A., Brittain, J.E. (1995). Radiocesium
in the sediments of Ovre Heimdalsvatn, a Norwegian subalpine lake. J.
Environ. Radioactivity, 27, 1-11.
Autumn 1990 |
Norway |
Stream substrate, organism |
137Cs |
190,000 kBq/kg (190,000,000 Bq/kg) |
Autumn 1990 |
Norway |
Stream gravel |
137Cs |
22,000 kBq/kg (22,000,000 Bq/kg) |
Autumn 1990 |
Norway |
Average sediment samples |
137Cs |
500 kBq/m2 (500,000 Bq/m2) |
-
"One sediment sample with 1,846 kBq/m2 (1,846,000
Bq/m2) was discarded." (pg. 6).
-
"... The radiocesium concentration increased with increasing
percentage of organic matter, water content, and with distance from the
main inlet.... the total radiocesium activity in the sediments may remain
unchanged or even increase during the years to come." (pg. 1).
Pacyna, J.M., Semb, A. and Christenson, G.C. (1989).
Migration
of 137Cs from air to soil and plants in the Gulsvik area, Norway
after the Chernobyl reactor accident. Report No. NILU-TR-2/88. Lillestroem,
Norsk Inst. for Luftforskning, Norway.
-
"Uptake of 137Cs from soil to plants through
their root system is not a rapid process... the effect of the Chernobyl
releases is not an acute but a long-term phenomenon." (Dialog abstract
quote).
Pinglot, J. F., Pourchet, M., Lefauconnier, B., Hagen,
J. O., Vaikmae, R., Punning, J. M., Watanabe, O., Takahashi, S. and Kameda,
T., (1994). Natural and artificial radioactivity in the Svalbard glaciers.
J.
Environ. Radioactivity. 25. pg. 161-176.
-
"Natural and artificial radioactivity in the snow of 10
Svalbard glaciers has been measured from 31 ice core samples, drilled between
1981 and 1993. Of these ice cores seven exhibit the well-known level arising
from the fallout of the 1961-62 atmospheric thermonuclear tests. The second
level, due to the Chernobyl accident (26 April 1986), has been detected
in all the studied glaciers; the maximum 137Cs fallout reaches
22 Bq kg-1 and shows a high variability." (pg. 161).
-
"The Chernobyl fallout is about 20Bq m-2 per
annum, similar to the value found in Greenland, and smaller than that found
in the French Alps (400 Bq m-2 per annum)." (pg. 174).
-
"The 137Cs fallout from the atmospheric thermonuclear
tests reaches about 10 to 20 times the Chernobyl fallout, at 200-540 Bq
m-2, at the deposition date." (pg. 174).
-
"The natural radioactivity (mainly 210Pb) is
higher than the artificial deposits, ... The fallout of 210Pb
since 1986 is about 5 times the deposit of 137Cs from Chernobyl."
(pg. 174).
Pourchet, M., Lefauconnier, B., Pinglot, J. F. and Hagen,
J. O. (1995). Mean net accumulation of ten glacier basins in Svalbard estimated
from detection of radioactive layers in shallow ice cores. Zeitschrift
fur Gletscherkunde und Glazialgeologie. 31. pg. 73 - 84.
-
"Present and recent past mean net accumulations are estimated
from the detection of dated radioactive layers in 31 shallow ice-cores
over ten glaciers in Svalbard. The reference layer due to fall-out of radioactive
elements after the Chernobyl accident has been detected in 25 ice cores
and gives a clear mark of the 1986 ablation surface. A layer corresponding
to fall-out from atmospheric nuclear tests conducted in 1961 and 1962 has
also been detected in eight ice cores." (pg. 73).
Solem, J.O. and Gaare, E. (1992). Radiocesium in aquatic
invertebrates from Dovrefjell, Norway, 1986 to 1989, after the Chernobyl
fall-out. J. Environ. Radioactivity. 17(1). pg. 1-12.
1985 |
Dovrefjell, Norway |
Reindeer Lichen, 5 samples |
137Cs |
350-450 Bq/kg |
1986 |
Dovrefjell, Norway |
Reindeer Lichen, 6 samples |
137Cs |
10,000 to 25,000 Bq/kg |
1986 |
Dovrefjell, Norway |
Ground deposition |
137Cs |
to 80,000 Bq/m2 |
1986 |
Dovrefjell, Norway |
Plankton feeders |
137Cs |
9,855 Bq/kg dry weight |
-
Contamination in aquatic invertebrates varied widely due
to patchy rainfall associated deposition.
-
Some samples showed an increase between 1988 and 1989.
Staaland, H., Garmo, T.H., Hove, K. and Pedersen, O. (1995).
Feed selection and radiocesium intake by reindeer, sheep and goats grazing
alpine summer habitats in southern Norway. J. Environ. Radioactivity.
29(1). pg. 39-56.
1987 |
Jotunheim, Norway |
Lichen |
137Cs |
40,040 Bq/kg dry weight |
1988 |
Jotunheim, Norway |
Moss |
137Cs |
20,290 Bq/kg dry weight |
1987 |
Jotunheim, Norway |
Moss |
137Cs |
40,180 Bq/kg dry weight |
-
Mean value of ground deposition in all grazing areas equaled
54,000 Bq m-2.
-
Depending on the type of vegetation in the grazed areas,
the transfer of radiocesium from soil to grazed vegetation (Bq kg-1
dry extrusa/Bq m-2 soil) was estimated to 0.02-0.04 in sheep,
0.02-0.05 in goats and 0.02-0.43 in reindeer for 1987. (pg. 39).
Steinnes, E. and Njastad, O. (1993). Use of mosses and
lichens for regional mapping of 137Cs fallout from the Chernobyl
accident. J. Environ. Radioactivity. 21(1). pg. 65-74.
1986 |
Norway |
Lichen (Cladonia stellaris) |
134,137Cs |
60,000 Bq/kg d.w. |
1986 |
Norway |
Moss (Hylocomium splendens) |
134,137Cs |
40,000 Bq/kg d.w. |
-
Concentration of cesium was much less in another lichen,
hylocomium
physodes, and was less in spruce forest due to absorption of cesium
by needles prior to deposition on lichen.
Strand, T. (1987). Doses to the Norwegian population
from naturally occurring radiation and from the Chernobyl fallout.
Doctoral Dissertation. National Institute of Radiation Hygiene, Oslo.
1986 |
Norway |
Reindeer meat |
134,137Cs |
100,000 Bq/kg |
1986 |
Norway |
Freshwater fish |
134,137Cs |
55,000 Bq/kg |
1986 |
Norway |
Goat's milk products |
134,137Cs |
4,200 Bq/kg |
1986 |
Norway |
Mutton |
134,137Cs |
15,000 Bq/kg |
-
The Norwegian survey used approximately 30,000 samples
on foodstuffs in the first year after the Chernobyl accident; the above
data are peak concentrations.
-
The estimated annual intake of radiocesium following the
Chernobyl accident for the average Norwegian consumer was 10,500 Bq.
Broda, R. (1987). Gamma spectroscopy analysis of hot
particles from the Chernobyl fallout. Acta Physica Polica. B18.
pg. 935-950.
Example of radioactive fallout composition in Krakow
- Poland. A soil sample of 0.5 cm layer was measured 1st of May. |
132Te - 29.3 kBq/m2 |
140Ba - 2.5 kBq/m2 |
132I - 25.7 kBq/m2 |
140La - 2.4 kBq/m2 |
131I - 23.6 kBq/m2 |
99Mo - 1.7 kBq/m2 |
129mTe - 8.0 kBq/m2 |
106Ru - 1.3 kBq/m2 |
103Ru - 6.1 kBq/m2 |
127Sb - 0.8 kBq/m2 |
137Cs - 5.2 kBq/m2 |
136Cs - 0.7 kBq/m2 |
134Cs - 2.7 kBq/m2 |
|
-
Ground level activity up to 360,000 Bq/m2 in
Kracow area; the above sample is from a less contaminated area of Kracow.
-
Numerous hot particles were found in both the Kracow and
Masurian Lakes regions. See the summary of the same citation in Hot
Particles above.
Jaworowski, Z. and Kownacka, L. (1988). Tropospheric and
stratospheric distributions of radioactive iodine and cesium after the
Chernobyl accident. J. Environ. Radioactivity. 6. pg. 145-150.
-
On April 30, 1986, Warsaw ground level air concentration
of 131I was 11.5 Bq/m3 (11,500,000 µBq).
Mietelski, J. W., Broda, R. and Sieniawski, J. (1988).
Long lived isotopes in the Chernobyl radioactive cloud at Kracow. J.
Radioanal. Nucl. Chem., Letters. 127(5). pg. 367-378.
-
Peak gross air contamination in Kracow reached 250 Bq/m3
on April 30, 1986. Little nuclide specific data available. Ruthenium hot
particles were observed.
Piasecki, E. (1987). Spatial distribution of radioactive
fallout in Poland. J. Radioanal. Nucl. Chem, Letters. 118(5). pg.
369-372.
-
Very large spatial and temporal variability of radioactive
fallout in Poland. Total beta measurements were made only with crude instrumentation.
Rich, V. (1986). Fallout pattern puzzles Poles. Nature.
322(28). pg. 765.
-
Many hot spots were noted measuring tens to hundreds of
meters across and exhibiting levels radioactivity ten times higher than
the surrounding area. Ruthenium was the predominant hot spot nuclide although
a few hot spots also had barium or lanthinum as the predominant nuclide.
Rich, V. (1986). Polish fallout underestimated. Nature.
324. (number and page unavailable).
-
Early official reports from Poland were very inaccurate.
Robbins, J.A. and Jasinski, A.W. (1995). Chernobyl fallout
radionuclides in Lake Sniardwy, Poland. J. Environ. Radioactivity.
26(2). pg. 157-184.
-
Total 137Cs loading of Lake Sniardwy estimated
at an average of 6,100 Bq m-2.
-
Approximate particles settling rate one meter per day.
-
" The average Activity with 137Cs in the flesh
of bream increased up to 120 times that of pre Chernobyl levels measured
in 1985. (Bream to 493 mBq/g)" (pg. 157-158).
Seaward, M.R.D., Heslop, J.A., Green, D. and Bylinska,
E. A. (1988). Recent levels of radionuclides in lichens from southwest
Poland with particular reference to 134Cs and 137Cs.
J.
Environ. Radioactivity. 7. pg. 123-129.
August 1986 |
SW Poland |
Lichen |
95Nb |
8,114 Bq/kg |
August 1986 |
SW Poland |
Lichen |
103Ru |
2,065 Bq/kg |
August 1986 |
SW Poland |
Lichen |
106Ru/106Rh |
16,570 Bq/kg |
August 1986 |
SW Poland |
Lichen |
134Cs |
18,263 Bq/kg |
August 1986 |
SW Poland |
Lichen |
137Cs |
36,630 Bq/kg |
August 1986 |
SW Poland |
Lichen |
144Ce |
18,500 Bq/kg |
-
August 1986 samples of Umbilicaria collected in SW Poland
showed significant increases in radioactivity over 1978-79 levels. Lichen
are highly efficient accumulators of radionuclides.
Skwarzec, B. and Bojanowski, R. (1992). Distribution of
plutonium in selected components of the Baltic ecosystem within the Polish
economic zone. J. Environ. Radioactivity. 15(3). pg. 249-264.
-
Average values of 239,240Pu in seawater: 5
mBq m-3 of which 70% constituted filterable forms (<0.45
µm).
-
Concentration levels of plutonium were one order of magnitude
greater per kilogram of dried specimens vs. wet weight concentration.
-
Total plutonium deposition ranged from 30 Bqm-2
to 98 Bq m-2 at three sampling locations.
-
The highest concentration of Pu in sediment were probably
due to the Vistula river, which delivered 192 MBq 239,240Pu
in 1989 to the Baltic Sea.
-
Little impact from Chernobyl plutonium, unlike Chernobyl
cesium.
-
The concentration factor range was 600-27,100 in benthic
animals and sea plants.
Carvalho, F.P. (1986). Radioactivity fallout in
Portugal following the Chernobyl accident. Laboratorio Nacional de
Engenharia e Tecnologia Industrial, Saracem, Portugal.
-
Almost none of the Chernobyl fallout reached Portugal
compared to the rest of Europe. Within the Azore Islands, peak values of
131I
in milk 1.5 Bq/l, and for 137Cs 19 Bq/l.
Pourchet, M., Melieres, M. A., Silvestru, E., Rajka,
G., Candaudap, F. and Carbonnel, J. P. (May 26-30, 1996). Radionuclides
in a cave sediment core from Ghetarul de sub Zgurasti (Romania). 14th
Intern. Symposium on Theoretical and Applied Karstology. Baile Herculane-
Romania.
-
"the transmission of pollution from the earth surface
to remote areas like underground cave is very effective. To our knowledge
it is the first time that such substantial contamination is revealed."
(pg. 1).
-
"The 137Cs inventory relative to nuclear tests
(estimated from the 90Sr deposit) has been measured at Vienna
(Austria) and is of 2.95 kBq.m-2.y-1. The Chernobyl
137Cs
deposition in Romania has been estimated at Cluj to be 4 kBq.m-2,
but shows in Romania a wide range of values from 0.2 to 8.5 kBq.m-8."
(pg. 2).
Abaturov, Y.D., Abaturov, A.V., Bykov, A.V., et al.
(1996).
The effect of ionizing irradiation on the pine forests in the
nearest zone of the Chernobyl nuclear power plant. ISBN 5-02-001918-6.
M. Nauka. pp. 140.
-
"Materials of researches in 1987-1992 over the territory adjacent to
Chernobyl nuclear power plant are generalized in the monograph. A three-dimensional
picture of area of irradiation damage of pine along the western trace of
radioactive fall-outs is presented. The most important elements of irradiation
situation during an active phase of the incident are reconstructed." (abstract).
AUIAR. Cs-137 and Cs-134 contamination map of Byelorussia
based on data from 1989. Byelorussian Department of the All Union Institute
for Agricultural Radiology, Gomel. (unpublished).
Cooper, E.L., Zeiller, E., Ghods-Esphahani, A., Makarewicz,
M., Schelenz, R., Frindik, O., Heilgeist, M. and Kalus, W. (1992). Radioactivity
in food and total diet samples collected in selected settlements in the
USSR. J. Environ. Radioactivity. 17(2+3). pg. 147-158.
1987 |
Novozybkov |
Wild blueberries |
137Cs |
1240 Bq/kg wet weight |
1987 |
Savici |
Mushroom |
137Cs |
131,000 Bq/kg wet weight |
1987 |
Daleta |
Total dietary intake per kg of food |
137Cs |
6,370 Bq/kg total diet average |
1987 |
Daleta |
Total dietary intake |
Total alpha |
1300 µBq/g (1.3 Bq/kg) dry weight |
-
Daleta, an area with the "lowest" surface contamination,
had 137Cs deposition levels of 1-5 Ci km2 (37,000
to 185,000 Bq/M2).
Egorov, Nikolai N., Novikov, Vladimir M., Parker, Frank
L. and Popov, Victor K., Eds. (June 2000). The radiation legacy of the
Soviet nuclear complex. Earthscan Publications Ltd., United Kingdom.
IS.
-
The annotations of this text are in
the section on Russian nuclear power plants.
Fleishman, D.G., Nikiforov, V.A., Saulus, A.A.
and Komov, V.T. (1992). 137Cs in fish of some lakes and rivers
of the Bryansk region and north-west Russia in 1990-1992. J. Environ.
Radioactivity. 24(2). pg. 145-158.
-
The highest levels of 137Cs ranged up to 15,000-21,000
Bq/kg wet weight. (pg. 145).
-
"Fish from lakes generally contained more 137Cs
(up to about ten times) than those from rivers, both in the heavily contaminated
zone and in the lightly contaminated regions." (pg. 145).
-
"Between 1990 and 1992 there was no significant general
decrease of 137Cs content in fish." (pg. 145).
Holliday, B., Binns, K.C. and Stewart, S.P. (1986). Monitoring
Minsk and Kiev students after Chernobyl. Nature. 321. pg. 820-821.
-
"Using published NRPB information, an acceptance level
with 30 Bq/cm2 (300,000 Bq/m2)... was adopted as
the clearance level for clothing contamination on returning students."
(pg. 820).
-
"Most of the clothing showed positive indications of contamination
but only 2% of the clothing monitored was in excess of the "clearance level."
(pg. 821).
-
Approximate thyroid radioactivity of 99 students reentering
to the United Kingdom ranged from 800 Bq to 6,900 Bq with a maximum calculated
intake on 26 April of 53,000 Bq.
IAEA (1990). The radiological consequences in the USSR
from the Chernobyl accident: Assessment of health and environmental effects
and evaluation of protective measures. Project description and scheme
of implementation as approved by the International Advisory Committee,
International Atomic Energy Agency report, and appendices. IAEA, Vienna.
Kliashtorn, A.L., Tikhomirov, F.A. and Shcheglov, A.I.
(1984). Lysimetrical study of radionuclides in the forests around the Chernobyl
nuclear power plant. J. Environ. Radioactivity. 24. pg. 81-90.
-
"Sum total accumulation deposition of the radionuclides
(Ce-144; Cs-134,137; Ru-106; Sr-90) ranged from 90 MBq/m2 to
0.5 Mbq/m2 (90,000,000 Bq/m2 - 500,000 Bq/m2)."
(pg. 81).
-
"It was shown that 0.01-0.6% of the total amount of radionuclides
was lost from the 20-30 cm layer of soil every year depending on the type
of radionuclide, type of ecosystem and the location of study plot." (pg.
207).
Knatko, V.A., Skomorokhov, A.G., Asimova, V.D., Strakh,
L.I., Bogdanov, A.P. and Mironov, V.P. (1996). Characteristics of 90Sr,
137Cs
and 239,240Pu migration in undisturbed soils of southern Belarus
after the Chernobyl accident. J. Environ. Radioactivity. 30(2).
pg. 185-196.
1994 |
Southern Belarus |
Total activity; soil horizon 0-20 cm. |
137Cs |
6,700,000 Bq/m2 |
1994 |
Southern Belarus |
Total activity; soil horizon 0-20 cm. |
239,240Pu |
37,700 Bq/m2 |
-
"These values are 102-103 times
higher than the global fallout." (pg. 189).
Knatko, V.A., Gurkov, V.V., Asimova, V.D., Shpakovskaya,
E.B. and Shimanovich, E.A. (1994). Soil-milk transfer of 137Cs
in an area of Byelorussia after the Chernobyl accident. J. Environ.
Radioactivity. 22(3). pg. 269-278.
-
"Some hundreds of kilometers from Chernobyl the level
of soil contamination varies over several orders of magnitude and is sometimes
higher than 1,000,000 Bq m-2." (pg. 269).
-
"TF (transfer) values decrease with increasing soil contamination
levels, except a constant TF value is achieved in highly contaminated soil."
(pg. 277).
Kryshev, I.I. (1995). Radioactive contamination of aquatic
ecosystems following the Chernobyl accident. J. Environ. Radioactivity.
27(3). pg. 207-220.
May 1986 |
Chernobyl |
Cooling pond sediments |
95Zr |
54,000,000 Bq/m2 |
May 1986 |
Chernobyl |
Cooling pond sediments |
95Nb |
50,000,000 Bq/m2 |
May 1986 |
Chernobyl |
Cooling pond sediments |
137Cs |
5,000,000 Bq/m2 |
May 1986 |
Chernobyl |
Cooling pond sediments |
144Ce |
40,000,000 Bq/m2 |
May 1986 |
Chernobyl |
Algae |
137Cs |
90,000 Bq/m2 |
1987 |
Chernobyl |
Pike muscle |
137Cs |
420,000 Bq/kg fresh weight |
1989 |
Kiev reservoir |
Mollusc |
90Sr |
1,200 Bq/kg fresh weight |
-
"The CNPP cooling pond... was formed by cutting off part
of the Pripyat River plain with a dike." (pg. 209).
-
"Reduction in the 137Cs concentration proceeded
slowly in most of the aquatic ecosystems." (pg. 207).
Likhtarev, I.A., Kovgan, L.N., Vavilov, S.E., Gluvchinsky,
R.R., Perevoznikov, O.N., Litvinets, L.N., Anspaugh, L.R., Kercher, J.R.
and Bouville, A. (1996). Internal exposure from the ingestion of foods
contaminated by 137Cs after the Chernobyl accident. Report 1.
General model: Ingestion doses and countermeasure effectiveness for the
adults of Rovno oblast of Ukraine. Health Physics. 70(3). pg. 297-317.
-
"Fallout of 137Cs in these regions [Rovno Oblast]
of Ukraine was lower than in other regions of Ukraine. However, the transfer
of 137Cs from soil to milk in the region considered is high
(up to 20 Bq L-1 per kBq m-2" (pg. 297).
Poiarkov, V.A., Nazarov, A.N. and Kaletnik, N.N. (1995).
Post-Chernobyl radiomonitoring of Ukrainian forest ecosystems. J. Environ.
Radioactivity. 26. pg. 259-271.
-
137Cs activities now measured in Ci km-2
in litter, and per 0-2 and 5 cm units of soil depth.
-
Peak concentration in litter: 12.3 Ci km-2
(1 Ci/km2=37,000 Bq/m2).
-
"The bulk of the activity occurs in the top 15 cm of the
soil profile... Soil Profiles indicate no substantial differences for 1991
and 1992 suggesting that 137Cs has a limited mobility." (pg.
259).
Polikarpov, G.G., Kulebakina, L.G., Timoshchuk, V.I. and
Stokozov, N.A. (1991). 90Sr and 137Cs in surface
waters of the Dnieper River, the Black Sea and the Aegean Sea in 1987 and
1988. J. Environ. Radioactivity 13(1). pg. 25-38.
-
Concentrations of 90Sr in the Dnieper River,
which drains the Pripjat River near Chernobyl, were up to ten times greater
than cesium concentrations, "probably due to the ability of cesium to become
absorbed on suspended particles... and the high solubility of strontium
in fresh water." (pg. 36).
Robertson, D.E., Perkins, R.W., Lepel, E.L. and Thomas,
C.W. (1992). Radionuclide concentrations in environmental samples collected
around Chernobyl during the International Chernobyl Project - analyses
conducted by Battelle, Pacific Northwest Laboratory. J. Environ. Radioactivity.
17(2+3). pg. 159-182.
1990 |
Svjatsk |
Creek sediment |
137Cs |
4.53 Bq/g |
1990 |
Soboli |
Rock moss scrapings |
137Cs |
552 Bq/g (552,000 Bq/kg) |
1990 |
Bragin |
Tombstone moss scrapings |
239,240Pu |
0.979 Bq/g (979 Bq/kg) |
1990 |
Bragin |
Soil core |
129I |
5.11 x 10-6Bq/g |
-
129I 1/2T = 15.9 million years.
-
"Moss species appear to be efficient collectors of the
Chernobyl fallout in this region." (pg. 159).
-
"Analyses of undisturbed soil cores indicated that the
Chernobyl fallout was still concentrated in the upper several centimeters
of soil as of August, 1990. Cesium-137 is the least mobile of all of the
radionuclides measured." (pg. 159).
Salbu, B., Oughton, D.H., Ratnikov, A.V., Zhigareva, T.L.,
Kruglov, S.V., Petrov, K.V., Grebenshakikova, N.V., Firsakova, S.K., Astasheva,
N.P., Loshchilov, N.A., Hove, K. and Strand, P. (1994). The mobility of
137Cs
and 90Sr in agricultural soils in the Ukraine, Belarus, and
Russia, 1991. Health Physics. 67(5). pg. 518-528.
-
"The sites, representing plowed and natural pastures,
were located at varying distances between 50 and 650 km and varying directions
from the Chernobyl reactor site." (pg. 518).
-
"The 137Cs activity concentrations in the upper
0-5 cm soil layer ranged from 25-1,000 kBqm-2 and were higher
in natural pastures as compared to plowed pastures." (pg. 518).
-
"For 90Sr, activity levels ranged from 1.4-40
kBq m-2" (pg. 518).
Steinhausler, F. (1992). Uncertainties associated with
the corroboration of official USSR environmental data in areas contaminated
by Chernobyl fallout. J. Environ. Radioactivity. 17(2+3). pg. 211-232.
1990 |
Bragin |
Lichen (Parmelia sulcata) |
137Cs |
326,000 Bq/kg |
-
"The results show that the uncertainty associated with
official data on 137Cs is relatively low." (pg. 211).
Tracy, B.L., Kramer, G.H. and Gamarnik, K. (1993). Radiocesium
in children from Belarus. Health Physics. 66(4). pg. 439-443.
-
"The body burdens of 137Cs were measured in
74 children from Belrus who had been exposed to fallout from the Chernobyl
accident...[who were]...visiting the Ottawa area during the summers of
1991 and 1992." (pg. 439).
-
"The body burdens were related to some extent, with recorded
fallout levels in the region of origin but did not appear to change significantly
from 1991 to 1992." (pg. 439).
-
"During their stay in Canada, radiocesium was being cleared
from the children's bodies with a mean half-time of 33 d (range= 12-77
d)." (pg. 439).
USSR State Committee on Hydrometeorology. (1991). Radiation
maps in the territory of the European part of the USSR as of December 1990.
Densities of area contamination by cesium-137, strontium-90, and plutonium-239,
240. SCH, Minsk.
van den Berg, G.J., Tyssen, T.P.M., Ammerlaan, M.J.J.,
Volkers, K.J., Woroniecka, U.D., de Bruin, M. and Wolterbeek, H. Th. (1992).
J.
Environ. Radioactivity. 17(2+3). pg. 115-128.
1986 |
Bragin |
Lichen |
137Cs |
1,630,000 Bq/kg |
-
"The lichen 137Cs levels are one to two orders
of magnitude higher than levels determined in 1986 in Poland, Greece or
the Netherlands." (pg. 115).
-
"Averaged lichen 137Cs levels (kBq kg-1)
are proportional to soil surface deposition (kBq m-2), except
for higher soil 137Cs activity classes (>500 kBqm-2),
where lichen data may lead to underestimates of actual deposition." (pg.
128).
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